Chemical adsorption enhanced CO2 capture and photoreduction over a copper porphyrin based metal organic framework

ACS Appl Mater Interfaces. 2013 Aug 14;5(15):7654-8. doi: 10.1021/am4019675. Epub 2013 Jul 12.

Abstract

Effective CO2 capture and activation is a prerequisite step for highly efficient CO2 reduction. In this study, we reported a case of Cu(2+) in a porphyrin based MOF promoted enhanced photocatalytic CO2 conversion to methanol. Compared with the sample without Cu(2+), the methanol evolution rate was improved as high as 7 times. In situ FT-IR results suggested that CO2 chemical adsorption and activation over Cu(2+) played an important role in improving the conversion efficiency.

Publication types

  • Research Support, Non-U.S. Gov't