MRI evidence for a receding-front effect in drying porous media

Phys Rev E Stat Nonlin Soft Matter Phys. 2013 Jun;87(6):062303. doi: 10.1103/PhysRevE.87.062303. Epub 2013 Jun 10.

Abstract

After drying colloidal particles suspended in a porous medium a concentration gradient appears. Using ^{1}H MRI we propose a protocol to observe simultaneously the distributions of air, liquid, and colloid through the unsaturated solid porous structure. Thus we show that the above phenomenon comes from a receding-front effect: The elements migrate towards the free surface of the sample and accumulate in the remaining liquid films. Our understanding of the process makes it possible to establish a simple model without diffusion predicting the drying rate and the concentration distribution in time, in excellent agreement with the experimental observations.

MeSH terms

  • Adsorption
  • Air / analysis*
  • Computer Simulation
  • Desiccation / methods*
  • Diffusion
  • Magnetic Resonance Imaging / methods*
  • Models, Chemical*
  • Models, Molecular*
  • Phase Transition
  • Porosity
  • Protons
  • Solutions / chemistry*

Substances

  • Protons
  • Solutions