Crystal structure of polymeric carbon nitride and the determination of its process-temperature-induced modifications

J Phys Condens Matter. 2013 Oct 2;25(39):395402. doi: 10.1088/0953-8984/25/39/395402. Epub 2013 Sep 3.

Abstract

Based on the arrangement of two-dimensional 'melon', we construct a unit cell for polymeric carbon nitride (PCN) synthesized via thermal polycondensation, whose theoretical diffraction powder pattern includes all major features measured in x-ray diffraction. With the help of this unit cell, we describe the process-temperature-induced crystallographic changes in PCN that occur within a temperature interval between 510 and 610 °C. We also discuss further potential modifications of the unit cell for PCN. It is found that both triazine- and heptazine-based g-C3N4 can only account for minor phases within the investigated synthesis products.

Publication types

  • Research Support, Non-U.S. Gov't