Lipid peroxidation is essential for phospholipase C activity and the inositol-trisphosphate-related Ca²⁺ signal

J Cell Sci. 2014 Jan 1;127(Pt 1):21-6. doi: 10.1242/jcs.138370. Epub 2013 Nov 6.

Abstract

Reactive oxygen species (ROS) are produced in enzymatic and non-enzymatic reactions and have important roles in cell signalling but also detrimental effects. ROS-induced damage has been implicated in a number of neurological diseases; however, antioxidant therapies targeting brain diseases have been unsuccessful. Such failure might be related to inhibition of ROS-induced signalling in the brain. Using direct kinetic measures of lipid peroxidation in astrocytes and measurements of lipid peroxidation products in brain tissue, we here show that phospholipase C (PLC) preferentially cleaves oxidised lipids. Because of this, an increase in the rate of lipid peroxidation leads to increased Ca(2+) release from endoplasmic reticulum (ER) stores in response to physiological activation of purinoreceptors with ATP. Both vitamin E and its water-soluble analogue Trolox, potent ROS scavengers, were able to suppress PLC activity, therefore dampening intracellular Ca(2+) signalling. This implies that antioxidants can compromise intracellular Ca(2+) signalling through inhibition of PLC, and that PLC plays a dual role - signalling and antioxidant defence.

Keywords: Astrocyte; Ca2+; Lipid peroxidation; Phospholipase C.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Adenosine Triphosphate / metabolism
  • Adenosine Triphosphate / pharmacology
  • Animals
  • Antioxidants / pharmacology
  • Astrocytes / cytology
  • Astrocytes / drug effects*
  • Astrocytes / metabolism
  • Calcium / metabolism*
  • Calcium Signaling / drug effects*
  • Cerebral Cortex / cytology
  • Cerebral Cortex / drug effects
  • Cerebral Cortex / metabolism
  • Chromans / pharmacology
  • Coculture Techniques
  • Endoplasmic Reticulum / drug effects
  • Endoplasmic Reticulum / metabolism
  • Hippocampus / cytology
  • Hippocampus / drug effects
  • Hippocampus / metabolism
  • Inositol 1,4,5-Trisphosphate / metabolism*
  • Lipid Metabolism / drug effects
  • Lipid Peroxidation
  • Male
  • Mesencephalon / cytology
  • Mesencephalon / drug effects
  • Mesencephalon / metabolism
  • Neurons / cytology
  • Neurons / drug effects*
  • Neurons / metabolism
  • Primary Cell Culture
  • Rats
  • Rats, Sprague-Dawley
  • Reactive Oxygen Species / antagonists & inhibitors
  • Reactive Oxygen Species / metabolism
  • Receptors, Purinergic
  • Type C Phospholipases / antagonists & inhibitors
  • Type C Phospholipases / metabolism*
  • Vitamin E / pharmacology

Substances

  • Antioxidants
  • Chromans
  • Reactive Oxygen Species
  • Receptors, Purinergic
  • Vitamin E
  • Inositol 1,4,5-Trisphosphate
  • Adenosine Triphosphate
  • Type C Phospholipases
  • 6-hydroxy-2,5,7,8-tetramethylchroman-2-carboxylic acid
  • Calcium