Synthesis of ¹⁸F-labelled β-lactams by using the Kinugasa reaction

Chemistry. 2014 Apr 14;20(16):4697-703. doi: 10.1002/chem.201304056. Epub 2014 Mar 11.

Abstract

Owing to their broad spectrum of biological activities and low toxicity, β-lactams are attractive lead structures for the design of novel molecular probes. However, the synthesis of positron emission tomography (PET)-isotope-labelled β-lactams has not yet been reported. Herein, we describe the simple preparation of radiofluorinated β-lactams by using the fast Kinugasa reaction between (18)F-labelled nitrone [(18)F]-1 and alkynes of different reactivity. Additionally, (18)F-labelled fused β-lactams were obtained through the reaction of a cyclic nitrone 7 with radiofluorinated alkynes [(18)F]-6 a,b. Radiochemical yields of the Kinugasa reaction products could be significantly increased by the use of different Cu(I) ligands, which additionally allowed a reduction in the amount of precursor and/or reaction time. Model radiofluorinated β-lactam-peptide and protein conjugates ([(18)F]-10 and (18)F-labelled BSA conjugate) were efficiently obtained in high yield under mild conditions (aq. MeCN, ambient temperature) within a short reaction time, demonstrating the suitability of the developed method for radiolabelling of sensitive molecules such as biopolymers.

Keywords: click chemistry; imaging agents; isotopic labelling; radiopharmaceuticals; β-lactams.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Alkynes / chemistry
  • Animals
  • Cattle
  • Click Chemistry
  • Contrast Media / chemical synthesis
  • Contrast Media / chemistry
  • Fluorine Radioisotopes / chemistry
  • Isotope Labeling
  • Nitrogen Oxides / chemistry
  • Positron-Emission Tomography
  • Radiopharmaceuticals / chemical synthesis
  • Radiopharmaceuticals / chemistry
  • Serum Albumin, Bovine / chemistry
  • beta-Lactams / chemical synthesis*
  • beta-Lactams / chemistry

Substances

  • Alkynes
  • Contrast Media
  • Fluorine Radioisotopes
  • Nitrogen Oxides
  • Radiopharmaceuticals
  • beta-Lactams
  • nitrones
  • Serum Albumin, Bovine