Adsorption of phthalic acid esters (PAEs) by amphiphilic polypropylene nonwoven from aqueous solution: the study of hydrophilic and hydrophobic microdomain

J Hazard Mater. 2014 May 30:273:61-9. doi: 10.1016/j.jhazmat.2014.03.029. Epub 2014 Mar 28.

Abstract

A kind of amphiphilic polypropylene nonwoven with hydrophilic and hydrophobic microdomain was prepared through electron beam induced graft polymerization and subsequent ring opening reaction and then utilized in the adsorption of phthalic acid esters (PAEs). To elucidate the superiority of such amphiphilic microdomain, a unique structure without hydrophilic part was constructed as comparison. In addition, the adsorption behaviors including adsorption kinetics, isotherms and pH effect were systematically investigated. The result indicated that the amphiphilic structure and the synergy between hydrophilic and hydrophobic microdomain could considerably improve the adsorption capacities, rate and affinity. Particularly the existence of hydrophilic microdomain could reduce the diffusion resistance and energy barrier in the adsorption process. These adsorption results showed that the amphiphilic PP nonwoven have the potential to be used in environmental application.

Keywords: Adsorption; Affinity; Diffusion resistance; Microdomain; Polypropylene; Synergy.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Adsorption
  • Amines / chemistry
  • Dibutyl Phthalate / chemistry*
  • Diethylhexyl Phthalate / chemistry*
  • Epoxy Compounds / chemistry
  • Esters
  • Hydrophobic and Hydrophilic Interactions
  • Methacrylates / chemistry
  • Polypropylenes / chemistry*
  • Solutions
  • Textiles
  • Water Pollutants, Chemical / chemistry*
  • Water Purification / methods

Substances

  • Amines
  • Epoxy Compounds
  • Esters
  • Methacrylates
  • Polypropylenes
  • Solutions
  • Water Pollutants, Chemical
  • Dibutyl Phthalate
  • Diethylhexyl Phthalate
  • glycidyl methacrylate
  • octylamine