Nanostructured weathering steel for matrix-free laser desorption ionisation mass spectrometry and imaging of metabolites, drugs and complex glycans

Analyst. 2014 Jun 7;139(11):2873-83. doi: 10.1039/c4an00216d.

Abstract

Weathering steel has been employed for the first time to prepare sample plates for matrix-free laser desorption ionisation mass spectrometry (LDI-MS) of small molecules up to a mass range of around 1500 Da. The effective UV absorption, heat conductivity and porosity of the nanostructured inner rust layer formed during passivation determine the excellent performance in LDI-MS for a broad range of different analyte classes. The inexpensive material was evaluated in a series of relevant analytical applications ranging from the matrix-free detection of serum metabolites, lactose quantification, lipid analysis in milk to the glycoprofiling of antibodies and imaging mass spectrometry of brain tissue samples.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Humans
  • Nanostructures*
  • Pharmaceutical Preparations / analysis*
  • Pharmaceutical Preparations / blood
  • Polysaccharides / analysis*
  • Polysaccharides / blood
  • Spectrometry, Mass, Matrix-Assisted Laser Desorption-Ionization / methods*
  • Spectrophotometry, Ultraviolet
  • Steel*

Substances

  • Pharmaceutical Preparations
  • Polysaccharides
  • Steel