Analgesic efficacy and safety of DALDA peptide analog delivery to the brain using oil-in-water nanoemulsion formulation

Pharm Res. 2014 Oct;31(10):2724-34. doi: 10.1007/s11095-014-1370-y. Epub 2014 May 3.

Abstract

Purpose: The main objective of this study was to develop and evaluate therapeutic efficacy and safety following systemic delivery of a peptide analgesic into the CNS using an oil-in-water nanoemulsion system.

Methods: We have formulated a safe and effective, omega-3 rich polyunsaturated fatty acid containing oil-in-water nanoemulsion formulation, for encapsulating and delivering chemically-modified DALDA, a potent mu-opioid peptide analogue, to the CNS. One of the challenges with CNS delivery is the lack of a non-invasive bioanalytical technique to confirm CNS uptake and therapeutic efficacy. Using blood oxygen-level dependent (BOLD) functional magenetic resonance imaging (fMRI), we provide quantitative evidence of nanoemulsion-based delivery and analgesic activity of DALDA analogue in capsaicin-induced awake rat model of pain.

Results: Nanoemulsion formulation effectively encapsulated the modified analgesic peptide and demonstrated efficacy in the capsaicin- pain induced functional magnetic resonance imaging model in rodents. Preliminary safety evaluations show that the nanoemulsion system was well tolerated and did not cause any acute negative effects.

Conclusions: Overall, these results show tremendous opportunity for the development of modified peptide analgesic-encapsulated nanoemulsion formulations for CNS delivery and therapeutic efficacy.

Publication types

  • Research Support, N.I.H., Extramural

MeSH terms

  • Analgesics / administration & dosage*
  • Analgesics / chemistry
  • Analgesics / pharmacokinetics
  • Analgesics / therapeutic use
  • Animals
  • Brain / drug effects*
  • Brain / metabolism
  • Brain / pathology
  • Capsaicin / pharmacology
  • Disease Models, Animal
  • Drug Carriers / chemistry*
  • Emulsions
  • Magnetic Resonance Imaging
  • Male
  • Mice, Inbred Strains
  • Nanostructures / chemistry*
  • Oligopeptides / administration & dosage*
  • Oligopeptides / chemistry
  • Oligopeptides / pharmacokinetics
  • Oligopeptides / therapeutic use
  • Pain / drug therapy
  • Pain / metabolism
  • Pain / pathology
  • Rats, Sprague-Dawley
  • Receptors, Opioid, mu / agonists*

Substances

  • Analgesics
  • Drug Carriers
  • Emulsions
  • Oligopeptides
  • Receptors, Opioid, mu
  • tyrosyl-arginyl-phenylalanyl-lysinamide
  • Capsaicin