[3+2] Photooxygenation of aryl cylopropanes via visible light photocatalysis

Tetrahedron. 2014 Jul 8;70(27-28):4270-4278. doi: 10.1016/j.tet.2014.02.045.

Abstract

We report that Ru(bpz)32+ is an excellent sensitizer for the photooxygenation of aryl cyclopropanes upon irradiation with visible light. The effectiveness of this photocatalyst enables the synthesis of a range of five-membered endoperoxides in excellent yield with quite low (0.5 mol%) catalyst loadings even when standard household light sources are utilized.

Keywords: Cyclopropanes; Endoperoxide; Photocatalysis; Photooxygenation; Radical cation.