Hubbard gap modulation in vanadium dioxide nanoscale tunnel junctions

Nano Lett. 2014 Nov 12;14(11):6115-20. doi: 10.1021/nl502065b. Epub 2014 Oct 16.

Abstract

We locally investigate the electronic transport through individual tunnel junctions containing a 10 nm thin film of vanadium dioxide (VO2) across its thermally induced phase transition. The insulator-to-metal phase transition in the VO2 film collapses the Hubbard gap (experimentally determined to be 0.4 ± 0.07 V), leading to several orders of magnitude change in tunnel conductance. We quantitatively evaluate underlying transport mechanisms via theoretical quantum mechanical transport calculations which show excellent agreement with the experimental results.

Keywords: Atomic force microscopy; density functional theory; metal−insulator transition; non-equilibrium Green’s function; tunnel junction; vanadium dioxide.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.