Transformation of cell-derived microparticles into quantum-dot-labeled nanovectors for antitumor siRNA delivery

Angew Chem Int Ed Engl. 2015 Jan 12;54(3):1036-40. doi: 10.1002/anie.201410223. Epub 2014 Nov 20.

Abstract

Cell-derived microparticles (MPs) have been recently recognized as critical intercellular information conveyors. However, further understanding of their biological behavior and potential application has been hampered by the limitations of current labeling techniques. Herein, a universal donor-cell-assisted membrane biotinylation strategy was proposed for labeling MPs by skillfully utilizing the natural membrane phospholipid exchange of their donor cells. This innovative strategy conveniently led to specific, efficient, reproducible, and biocompatible quantum dot (QD) labeling of MPs, thereby reliably conferring valuable traceability on MPs. By further loading with small interference RNA, QD-labeled MPs that had inherent cell-targeting and biomolecule-conveying ability were successfully employed for combined bioimaging and tumor-targeted therapy. This study provides the first reliable and biofriendly strategy for transforming biogenic MPs into functionalized nanovectors.

Keywords: biogenic vesicles; cell-derived microparticles; nanoparticles; quantum dots; targeted delivery.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Antineoplastic Agents / chemistry*
  • Antineoplastic Agents / metabolism
  • Antineoplastic Agents / therapeutic use
  • Apoptosis
  • Biotinylation
  • Cell Line, Tumor
  • Cell Proliferation
  • Cell-Derived Microparticles / chemistry*
  • Drug Carriers / chemistry
  • Fluoresceins / chemistry
  • Fluorescent Dyes / chemistry
  • Human Umbilical Vein Endothelial Cells
  • Humans
  • Mice
  • Mice, Nude
  • Microscopy, Fluorescence
  • Nanoparticles / chemistry
  • Neoplasms / diagnosis
  • Neoplasms / drug therapy
  • Quantum Dots / chemistry*
  • RNA, Small Interfering / chemistry*
  • RNA, Small Interfering / metabolism
  • RNA, Small Interfering / therapeutic use
  • Streptavidin / chemistry
  • Succinimides / chemistry
  • Transplantation, Heterologous
  • Vascular Endothelial Growth Factor A / antagonists & inhibitors
  • Vascular Endothelial Growth Factor A / genetics
  • Vascular Endothelial Growth Factor A / metabolism

Substances

  • 5-(6)-carboxyfluorescein diacetate succinimidyl ester
  • Antineoplastic Agents
  • Drug Carriers
  • Fluoresceins
  • Fluorescent Dyes
  • RNA, Small Interfering
  • Succinimides
  • Vascular Endothelial Growth Factor A
  • Streptavidin