Chip-based free-flow electrophoresis with integrated nanospray mass-spectrometry

Angew Chem Int Ed Engl. 2015 Feb 23;54(9):2766-70. doi: 10.1002/anie.201409663. Epub 2015 Jan 21.

Abstract

Free-flow electrophoresis is an ideal tool for preparative separations in continuous microflow. With the approach presented herein for coupling free-flow electrophoresis and mass spectrometry it is now also possible to trace non-fluorescent compounds and identify them by means of mass spectrometry. The functionality of the method and its potential as an integrated separation unit for microflow synthesis is demonstrated by application to a multicomponent [3+2]-cycloannulation.

Keywords: continuous micro flow-through; cycloaddition; electrophoresis; mass spectrometry; microfluidics.

MeSH terms

  • Benzaldehydes / chemical synthesis
  • Benzaldehydes / chemistry
  • Cyclization
  • Electrophoresis / methods*
  • Mass Spectrometry*
  • Molecular Structure
  • Nanotechnology*
  • Organosilicon Compounds / chemical synthesis
  • Organosilicon Compounds / chemistry
  • ortho-Aminobenzoates / chemical synthesis
  • ortho-Aminobenzoates / chemistry

Substances

  • Benzaldehydes
  • Organosilicon Compounds
  • ortho-Aminobenzoates
  • anthranilic acid
  • benzaldehyde