Abstract
Notch receptors guide mammalian cell fate decisions by engaging the proteins Jagged and Delta-like (DLL). The 2.3 angstrom resolution crystal structure of the interacting regions of the Notch1-DLL4 complex reveals a two-site, antiparallel binding orientation assisted by Notch1 O-linked glycosylation. Notch1 epidermal growth factor-like repeats 11 and 12 interact with the DLL4 Delta/Serrate/Lag-2 (DSL) domain and module at the N-terminus of Notch ligands (MNNL) domains, respectively. Threonine and serine residues on Notch1 are functionalized with O-fucose and O-glucose, which act as surrogate amino acids by making specific, and essential, contacts to residues on DLL4. The elucidation of a direct chemical role for O-glycans in Notch1 ligand engagement demonstrates how, by relying on posttranslational modifications of their ligand binding sites, Notch proteins have linked their functional capacity to developmentally regulated biosynthetic pathways.
Copyright © 2015, American Association for the Advancement of Science.
Publication types
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Research Support, N.I.H., Extramural
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Research Support, Non-U.S. Gov't
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Research Support, U.S. Gov't, Non-P.H.S.
MeSH terms
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Alagille Syndrome / genetics
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Amino Acid Sequence
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Amino Acid Substitution
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Animals
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Cell Line
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Conserved Sequence
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Crystallography, X-Ray
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Fucose / chemistry
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Glucose / chemistry
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Glycosylation
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Intracellular Signaling Peptides and Proteins / chemistry*
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Intracellular Signaling Peptides and Proteins / genetics
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Ligands
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Membrane Proteins / chemistry*
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Membrane Proteins / genetics
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Membrane Proteins / ultrastructure
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Molecular Sequence Data
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Molecular Targeted Therapy
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Polysaccharides / chemistry
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Precursor T-Cell Lymphoblastic Leukemia-Lymphoma / drug therapy
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Precursor T-Cell Lymphoblastic Leukemia-Lymphoma / genetics
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Protein Binding
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Protein Structure, Tertiary
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Rats
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Receptor, Notch1 / chemistry*
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Receptor, Notch1 / genetics
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Receptor, Notch1 / ultrastructure
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Serine / chemistry
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Serine / genetics
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Threonine / chemistry
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Threonine / genetics
Substances
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Intracellular Signaling Peptides and Proteins
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Ligands
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Membrane Proteins
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Notch1 protein, rat
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Polysaccharides
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Receptor, Notch1
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delta protein
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Fucose
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Threonine
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Serine
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Glucose