Quantitative analysis of the TNF-α-induced phosphoproteome reveals AEG-1/MTDH/LYRIC as an IKKβ substrate

Nat Commun. 2015 Apr 7:6:6658. doi: 10.1038/ncomms7658.

Abstract

The inhibitor of the nuclear factor-κB (IκB) kinase (IKK) complex is a key regulator of the canonical NF-κB signalling cascade and is crucial for fundamental cellular functions, including stress and immune responses. The majority of IKK complex functions are attributed to NF-κB activation; however, there is increasing evidence for NF-κB pathway-independent signalling. Here we combine quantitative mass spectrometry with random forest bioinformatics to dissect the TNF-α-IKKβ-induced phosphoproteome in MCF-7 breast cancer cells. In total, we identify over 20,000 phosphorylation sites, of which ∼1% are regulated up on TNF-α stimulation. We identify various potential novel IKKβ substrates including kinases and regulators of cellular trafficking. Moreover, we show that one of the candidates, AEG-1/MTDH/LYRIC, is directly phosphorylated by IKKβ on serine 298. We provide evidence that IKKβ-mediated AEG-1 phosphorylation is essential for IκBα degradation as well as NF-κB-dependent gene expression and cell proliferation, which correlate with cancer patient survival in vivo.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Blotting, Western
  • Cell Adhesion Molecules / drug effects*
  • Cell Adhesion Molecules / metabolism
  • Chromatin Immunoprecipitation
  • Chromatography, Liquid
  • Gene Expression Regulation, Neoplastic*
  • HEK293 Cells
  • Humans
  • I-kappa B Kinase / drug effects*
  • I-kappa B Kinase / metabolism
  • I-kappa B Proteins
  • Immunoprecipitation
  • MCF-7 Cells
  • Mass Spectrometry
  • Membrane Proteins
  • NF-KappaB Inhibitor alpha
  • NF-kappa B
  • Phosphoproteins
  • Phosphorylation / drug effects*
  • RNA-Binding Proteins
  • Serine
  • Tumor Necrosis Factor-alpha / pharmacology*
  • Tumor Stem Cell Assay
  • Up-Regulation

Substances

  • Cell Adhesion Molecules
  • I-kappa B Proteins
  • MTDH protein, human
  • Membrane Proteins
  • NF-kappa B
  • NFKBIA protein, human
  • Phosphoproteins
  • RNA-Binding Proteins
  • Tumor Necrosis Factor-alpha
  • NF-KappaB Inhibitor alpha
  • Serine
  • I-kappa B Kinase
  • IKBKB protein, human