Protection of coronary endothelial cells from cigarette smoke-induced oxidative stress by a new Mn(II)-containing polyamine-polycarboxilate scavenger of superoxide anion

Vascul Pharmacol. 2015 Dec:75:19-28. doi: 10.1016/j.vph.2015.06.008. Epub 2015 Jun 22.

Abstract

Oxidative stress plays a major role in cardiovascular injury and dysfunction induced by cigarette smoke. Smoke-borne pro-oxidants impair endothelial function and predispose to thrombosis, inflammation and atherosclerosis. This in vitro study evaluates whether Mn(II)(4,10-dimethyl-1,4,7,10-tetraazacyclododecane-1,7-diacetate).2H2O (Mn(II)(Me2DO2A)), a polyamine-polycarboxilate, Mn(II)-containing O2(-) scavenger, has a direct protective action on guinea pig coronary endothelial (GPCE) cells exposed to cigarette smoke extracts (CSE). Mn(II)(Me2DO2A) (1-10μmol/l) was added to the culture medium together with CSE and maintained for 4h. In parallel experiments, the inactive congener Zn(II)(Me2DO2A), in which Zn(II) replaced the functional Mn(II) center in the same organic scaffold, was used as negative control. Mn(II)(Me2DO2A), mostly at the higher doses (5 and 10μmol/l), significantly increased GPCE cell viability (trypan blue assay), improved mitochondrial activity (MTT test, mitochondrial membrane potential Δψ), reduced cellular apoptosis (mPTP, caspase-3 activity, TUNEL assay), decreased intracellular ROS levels (H2DCFDA), lipoperoxidation (BODIPY 581/591) and decreased protein nitrosylation. Of note, Zn(II)(Me2DO2A) did not preserve cell viability. These findings suggest that Mn(II)(Me2DO2A) is a promising O2(-) scavenging compound able to protect from cigarette smoke-induced oxidative cell injury. In perspective, should its efficacy be confirmed in future in vivo studies, this molecule might represent a therapeutic or preventive drug to counteract cigarette smoke toxicity.

Keywords: Cigarette smoke; Guinea pig coronary endothelial cells; Oxidative stress; ROS scavenger; Superoxide anion.

Publication types

  • Comparative Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Apoptosis / drug effects
  • Cell Survival / drug effects
  • Coronary Vessels / drug effects
  • Coronary Vessels / metabolism
  • Dose-Response Relationship, Drug
  • Endothelial Cells / drug effects
  • Endothelial Cells / metabolism
  • Free Radical Scavengers / administration & dosage
  • Free Radical Scavengers / pharmacology*
  • Guinea Pigs
  • In Vitro Techniques
  • Membrane Potential, Mitochondrial / drug effects
  • Mitochondria / metabolism
  • Organometallic Compounds / administration & dosage
  • Organometallic Compounds / pharmacology*
  • Oxidative Stress / drug effects*
  • Smoke / adverse effects*
  • Superoxides / metabolism

Substances

  • Free Radical Scavengers
  • Organometallic Compounds
  • Smoke
  • manganese(II) 4,10-dimethyl-1,4,7,10-tetraazacyclododecane-1,7-diacetate
  • Superoxides