High Concentrations of the Antibiotic Spiramycin in Wastewater Lead to High Abundance of Ammonia-Oxidizing Archaea in Nitrifying Populations

Environ Sci Technol. 2015 Aug 4;49(15):9124-32. doi: 10.1021/acs.est.5b01293. Epub 2015 Jul 21.

Abstract

To evaluate the potential effects of antibiotics on ammonia-oxidizing microbes, multiple tools including quantitative PCR (qPCR), 454-pyrosequencing, and a high-throughput functional gene array (GeoChip) were used to reveal the distribution of ammonia-oxidizing archaea (AOA) and archaeal amoA (Arch-amoA) genes in three wastewater treatment systems receiving spiramycin or oxytetracycline production wastewaters. The qPCR results revealed that the copy number ratios of Arch-amoA to ammonia-oxidizing bacteria (AOB) amoA genes were the highest in the spiramycin full-scale (5.30) and pilot-scale systems (1.49 × 10(-1)), followed by the oxytetracycline system (4.90 × 10(-4)), with no Arch-amoA genes detected in the control systems treating sewage or inosine production wastewater. The pyrosequencing result showed that the relative abundance of AOA affiliated with Thaumarchaeota accounted for 78.5-99.6% of total archaea in the two spiramycin systems, which was in accordance with the qPCR results. Mantel test based on GeoChip data showed that Arch-amoA gene signal intensity correlated with the presence of spiramycin (P < 0.05). Antibiotics explained 25.8% of variations in amoA functional gene structures by variance partitioning analysis. This study revealed the selection of AOA in the presence of high concentrations of spiramycin in activated sludge systems.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Ammonia / metabolism*
  • Anti-Bacterial Agents / analysis*
  • Archaea / genetics
  • Archaea / metabolism*
  • Bacteria / genetics
  • Bacteria / metabolism
  • Genes, Archaeal
  • Genetic Variation
  • Nitrification*
  • Nitrogen Cycle
  • Oxidation-Reduction
  • Phylogeny
  • Real-Time Polymerase Chain Reaction
  • Sequence Analysis, DNA
  • Sewage / microbiology
  • Spiramycin / analysis*
  • Wastewater / chemistry*
  • Wastewater / microbiology
  • Water Pollutants, Chemical / analysis*
  • Water Quality

Substances

  • Anti-Bacterial Agents
  • Sewage
  • Waste Water
  • Water Pollutants, Chemical
  • Ammonia
  • Spiramycin