Protonation effect on ligands in EuL: a luminescent switcher for fast naked-eye detection of HCl

Dalton Trans. 2015 Aug 14;44(30):13586-91. doi: 10.1039/c5dt01791b.

Abstract

A new luminescent coordination polymer, EuH(L)(2)(NO(3))(2) (EuL, HL = 2-(2-pyridin-2-yl)quinoline-4-carboxylic acid), has been solvothermally synthesized, and its framework of uncoordinated pyridyl rings was exploited for the binding and specific sensing of HCl via a protonation effect. The protonation effect changes the energy of the excited state of the ligands, rendering them unable to act as efficient antennae for Eu(3+) characteristic emission. Thus, we have developed a new, fast and convenient sensor for HCl, a gas harmful for the environment.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Coordination Complexes / chemistry*
  • Crystallography, X-Ray
  • Europium / chemistry*
  • Gases / analysis*
  • Hydrochloric Acid / analysis*
  • Ligands
  • Luminescence
  • Luminescent Measurements
  • Models, Molecular
  • Polymers / chemistry
  • Protons
  • Pyridines / chemistry*
  • Quinolines / chemistry*

Substances

  • Coordination Complexes
  • Gases
  • Ligands
  • Polymers
  • Protons
  • Pyridines
  • Quinolines
  • Europium
  • quinoline-4-carboxylic acid
  • Hydrochloric Acid