Evaluation of glycine-bearing celecoxib derivatives as a colon-specific mutual prodrug acting on nuclear factor-κB, an anti-inflammatory target

Drug Des Devel Ther. 2015 Aug 7:9:4227-37. doi: 10.2147/DDDT.S88543. eCollection 2015.

Abstract

In an inflammatory state where HOCl is generated, glycine readily reacts with HOCl to produce glycine chloramine, an anti-inflammatory oxidant. Colonic delivery of celecoxib elicits anticolitic effects in a trinitrobenzene sulfonic acid-induced rat colitis model. Glycine-bearing celecoxib derivatives were prepared and evaluated as a colon-specific mutual prodrug acting on nuclear factor-κB (NFκB), an anticolitic target. Glycylcelecoxib (GC), N-glycylaspart-1-ylcelecoxib (N-GA1C), and C-glycylaspart-1-ylcelecoxib (C-GA1C) were synthesized and their structures identified using infrared and proton nuclear magnetic resonance spectrometer. The celecoxib derivatives were chemically stable in pH 6.8 and 1.2 buffers. GC and C-GA1C were resistant to degradation in the small intestinal contents, while N-GA1C was substantially cleaved to release celecoxib. In contrast, all the celecoxib derivatives were degraded to liberate celecoxib in the cecal content. These results suggest that GC and C-GA1C could be delivered to and liberate celecoxib and glycine in the large intestine. In human colon carcinoma HCT116 and murine macrophage RAW264.7 cells, combined celecoxib-glycine chloramine treatment additively suppressed the production of proinflammatory NFκB target gene products. Collectively, our data suggest that C-GA1C is a potential colon-specific mutual prodrug acting against NFκB.

Keywords: celecoxib; colon-specific drug delivery; glycine chloramine; mutual prodrug; nuclear factor kappa-B.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Anti-Inflammatory Agents / chemical synthesis
  • Anti-Inflammatory Agents / chemistry
  • Anti-Inflammatory Agents / pharmacology*
  • Celecoxib / chemical synthesis
  • Celecoxib / chemistry
  • Celecoxib / pharmacology*
  • Cell Line
  • Colitis / drug therapy
  • Colon / metabolism*
  • Drug Delivery Systems
  • Drug Stability
  • Glycine / chemistry*
  • HCT116 Cells
  • Humans
  • Hydrogen-Ion Concentration
  • Inflammation / drug therapy
  • Macrophages / drug effects
  • Macrophages / metabolism
  • Male
  • Mice
  • NF-kappa B / metabolism
  • Prodrugs / chemical synthesis
  • Prodrugs / chemistry
  • Prodrugs / pharmacology
  • Rats
  • Rats, Sprague-Dawley

Substances

  • Anti-Inflammatory Agents
  • NF-kappa B
  • Prodrugs
  • Celecoxib
  • Glycine