Cloning, expression, purification and application of a novel chitinase from a thermophilic marine bacterium Paenibacillus barengoltzii

Food Chem. 2016 Feb 1:192:1041-8. doi: 10.1016/j.foodchem.2015.07.092. Epub 2015 Jul 23.

Abstract

A novel chitinase gene (PbChi70) from a marine bacterium Paenicibacillus barengoltzii was cloned and functionally expressed in Escherichia coli. The recombinant enzyme (PbChi70) was purified to homogeneity with a recovery yield of 51.9%. The molecular mass of purified enzyme was estimated to be 70.0 kDa by SDS-PAGE. PbChi70 displayed maximal activity at pH 5.5 and 55 °C, respectively. It exhibited strict substrate specificity for colloidal chitin, glycol chitin, powdery chitin, and N-acetyl chitooligosaccharides with degrees of polymerization above three. The enzyme exhibited an endo-type cleavage pattern and hydrolyzed colloidal chitin to yield mainly (GlcNAc)2. Furthermore, colloidal chitin was hydrolyzed by PbChi70 to produce 21.6 mg mL(-1) (GlcNAc)2 with the highest conversion yield of 89.5% (w/w). (GlcNAc)2 was further separated by an active charcoal column with a purity of 99% and a final yield of 61%. The unique enzymatic properties of the chitinase may make it a good candidate for (GlcNAc)2 production.

Keywords: Characterization; Chitin; Chitinase; Gene cloning; N-Acetyl chitobiose production; Paenicibacillus barengoltzii.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acetylglucosamine / metabolism
  • Chitin / analogs & derivatives
  • Chitin / metabolism
  • Chitinases / chemistry
  • Chitinases / genetics*
  • Chitinases / metabolism
  • Chitosan
  • Cloning, Molecular*
  • Escherichia coli / metabolism
  • Gene Expression*
  • Molecular Weight
  • Oligosaccharides
  • Paenibacillus / enzymology*
  • Recombinant Proteins / chemistry
  • Recombinant Proteins / metabolism
  • Substrate Specificity

Substances

  • Oligosaccharides
  • Recombinant Proteins
  • oligochitosan
  • Chitin
  • Chitosan
  • glycolchitin
  • Chitinases
  • Acetylglucosamine