Tellurium-Assisted Low-Temperature Synthesis of MoS2 and WS2 Monolayers

ACS Nano. 2015 Dec 22;9(12):11658-66. doi: 10.1021/acsnano.5b05594. Epub 2015 Nov 3.

Abstract

Chemical vapor deposition (CVD) is a scalable method able to synthesize MoS2 and WS2 monolayers. In this work, we reduced the synthesis temperature by 200 °C only by introducing tellurium (Te) into the CVD process. The as-synthesized MoS2 and WS2 monolayers show high phase purity and crystallinity. The optical and electrical performance of these materials is comparable to those synthesized at higher temperatures. We believe this work will accelerate the industrial synthesis of these semiconducting monolayers.

Keywords: chemical vapor deposition; molybdenum disulfide; transition metal dichalcogenides; tungsten disulfide; two-dimensional materials.

Publication types

  • Research Support, U.S. Gov't, Non-P.H.S.