Intermolecular Interactions and Protein Dynamics by Solid-State NMR Spectroscopy

Angew Chem Int Ed Engl. 2015 Dec 14;54(51):15374-8. doi: 10.1002/anie.201509168. Epub 2015 Nov 2.

Abstract

Understanding the dynamics of interacting proteins is a crucial step toward describing many biophysical processes. Here we investigate the backbone dynamics for protein GB1 in two different assemblies: crystalline GB1 and the precipitated GB1-antibody complex with a molecular weight of more than 300 kDa. We perform these measurements on samples containing as little as eight nanomoles of GB1. From measurements of site-specific (15) N relaxation rates including relaxation dispersion we obtain snapshots of dynamics spanning nine orders of magnitude in terms of the time scale. A comparison of measurements for GB1 in either environment reveals that while many of the dynamic features of the protein are conserved between them (in particular for the fast picosecond-nanosecond motions), much greater differences occur for slow motions with motions in the >500 ns range being more prevalent in the complex. The data suggest that GB1 can potentially undergo a small-amplitude overall anisotropic motion sampling the interaction interface in the complex.

Keywords: NMR spectroscopy; magic-angle spinning; protein dynamics; protein-antibody complexes; protein-protein interactions.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Nuclear Magnetic Resonance, Biomolecular / methods*
  • Protein Binding
  • Proteins / chemistry*

Substances

  • Proteins