Ligand Surface Chemistry Dictates Light Emission from Nanocrystals

J Phys Chem Lett. 2015 Nov 5;6(21):4292-6. doi: 10.1021/acs.jpclett.5b02015. Epub 2015 Oct 14.

Abstract

There are several contradictory accounts of the changes to the emissive behavior of semiconductor nanocrystal upon a ligand exchange from trioctylphosphine/cadmium-phosphonates passivation to N-butylamine. This communication explains the contradictory accounts of this reaction using new insights into ligand chemistry. Also, a previously unknown link between surface emission and cadmium-phosphonate (Z-type) ligands is shown.

Keywords: ligand; n-butylamine; nanocrystal; phosphonate.