p21-activated kinase group II small compound inhibitor GNE-2861 perturbs estrogen receptor alpha signaling and restores tamoxifen-sensitivity in breast cancer cells

Oncotarget. 2015 Dec 22;6(41):43853-68. doi: 10.18632/oncotarget.6081.

Abstract

Estrogen receptor alpha (ERα) is highly expressed in most breast cancers. Consequently, ERα modulators, such as tamoxifen, are successful in breast cancer treatment, although tamoxifen resistance is commonly observed. While tamoxifen resistance may be caused by altered ERα signaling, the molecular mechanisms regulating ERα signaling and tamoxifen resistance are not entirely clear. Here, we found that PAK4 expression was consistently correlated to poor patient outcome in endocrine treated and tamoxifen-only treated breast cancer patients. Importantly, while PAK4 overexpression promoted tamoxifen resistance in MCF-7 human breast cancer cells, pharmacological treatment with a group II PAK (PAK4, 5, 6) inhibitor, GNE-2861, sensitized tamoxifen resistant MCF-7/LCC2 breast cancer cells to tamoxifen. Mechanistically, we identified a regulatory positive feedback loop, where ERα bound to the PAK4 gene, thereby promoting PAK4 expression, while PAK4 in turn stabilized the ERα protein, activated ERα transcriptional activity and ERα target gene expression. Further, PAK4 phosphorylated ERα-Ser305, a phosphorylation event needed for the PAK4 activation of ERα-dependent transcription. In conclusion, PAK4 may be a suitable target for perturbing ERα signaling and tamoxifen resistance in breast cancer patients.

Keywords: ERα; PAK4; phosphorylation; small molecule inhibitor; tamoxifen resistance.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Benzimidazoles / pharmacology*
  • Breast Neoplasms / metabolism*
  • Breast Neoplasms / mortality
  • Breast Neoplasms / pathology
  • Databases, Genetic
  • Drug Resistance, Neoplasm / drug effects*
  • Drug Resistance, Neoplasm / physiology
  • Enzyme Inhibitors / pharmacology*
  • Estrogen Receptor alpha / metabolism*
  • Female
  • Flow Cytometry
  • Humans
  • Immunoblotting
  • Kaplan-Meier Estimate
  • MCF-7 Cells
  • Polymerase Chain Reaction
  • Pyrimidines / pharmacology*
  • RNA, Small Interfering
  • Selective Estrogen Receptor Modulators / pharmacology
  • Signal Transduction / physiology
  • Tamoxifen / pharmacology
  • Transfection
  • p21-Activated Kinases / metabolism*

Substances

  • 1-(2-(1-(2-aminopyrimidin-4-yl)-2-((2-methoxyethyl)amino)-1H-1,3-benzodiazol-6-yl)ethynyl)cyclohexan-1-ol
  • Benzimidazoles
  • ESR1 protein, human
  • Enzyme Inhibitors
  • Estrogen Receptor alpha
  • Pyrimidines
  • RNA, Small Interfering
  • Selective Estrogen Receptor Modulators
  • Tamoxifen
  • PAK4 protein, human
  • p21-Activated Kinases