O-GlcNAcylation of protein kinase A catalytic subunits enhances its activity: a mechanism linked to learning and memory deficits in Alzheimer's disease

Aging Cell. 2016 Jun;15(3):455-64. doi: 10.1111/acel.12449. Epub 2016 Feb 3.

Abstract

Alzheimer's disease (AD) is characterized clinically by memory loss and cognitive decline. Protein kinase A (PKA)-CREB signaling plays a critical role in learning and memory. It is known that glucose uptake and O-GlcNAcylation are reduced in AD brain. In this study, we found that PKA catalytic subunits (PKAcs) were posttranslationally modified by O-linked N-acetylglucosamine (O-GlcNAc). O-GlcNAcylation regulated the subcellular location of PKAcα and PKAcβ and enhanced their kinase activity. Upregulation of O-GlcNAcylation in metabolically active rat brain slices by O-(2-acetamido-2-deoxy-d-glucopyranosylidenamino) N-phenylcarbamate (PUGNAc), an inhibitor of N-acetylglucosaminidase, increased the phosphorylation of tau at the PKA site, Ser214, but not at the non-PKA site, Thr205. In contrast, in rat and mouse brains, downregulation of O-GlcNAcylation caused decreases in the phosphorylation of CREB at Ser133 and of tau at Ser214, but not at Thr205. Reduction in O-GlcNAcylation through intracerebroventricular injection of 6-diazo-5-oxo-l-norleucine (DON), the inhibitor of glutamine fructose-6-phosphate amidotransferase, suppressed PKA-CREB signaling and impaired learning and memory in mice. These results indicate that in addition to cAMP and phosphorylation, O-GlcNAcylation is a novel mechanism that regulates PKA-CREB signaling. Downregulation of O-GlcNAcylation suppresses PKA-CREB signaling and consequently causes learning and memory deficits in AD.

Keywords: Alzheimer's disease; O-GlcNAcylation; learning and memory; protein kinase A.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acetylglucosamine / metabolism*
  • Alzheimer Disease / pathology
  • Animals
  • Brain / drug effects
  • Brain / enzymology
  • Cyclic AMP Response Element-Binding Protein / metabolism
  • Cyclic AMP-Dependent Protein Kinase Catalytic Subunits / metabolism*
  • Diazooxonorleucine / pharmacology
  • Down-Regulation / drug effects
  • Glycosylation / drug effects
  • HEK293 Cells
  • HeLa Cells
  • Humans
  • Learning* / drug effects
  • Male
  • Memory / drug effects
  • Memory Disorders / pathology*
  • Mice, Inbred C57BL
  • Phosphorylation / drug effects
  • Protein Transport / drug effects
  • Rats, Sprague-Dawley
  • Subcellular Fractions / drug effects
  • Subcellular Fractions / enzymology
  • tau Proteins / metabolism

Substances

  • Cyclic AMP Response Element-Binding Protein
  • tau Proteins
  • Diazooxonorleucine
  • Cyclic AMP-Dependent Protein Kinase Catalytic Subunits
  • Acetylglucosamine