Investigating the Reactivity of 1,4-Anthracene-Incorporated Cycloparaphenylene

Org Lett. 2016 Apr 1;18(7):1574-7. doi: 10.1021/acs.orglett.6b00430. Epub 2016 Mar 22.

Abstract

Cycloparaphenylenes (CPPs) and their derivatives are unique conjugated macrocycles with novel optoelectronic and host-guest properties. A better understanding of their reactivity is essential for creating new functional materials utilizing these strained aromatic molecules as building blocks. 1,4-Anthracene-incorporated CPP 1 was synthesized and exhibited Diels-Alder reactivity but was unable to photodimerize. Comparison studies with cyclophane 2 and unstrained 3 indicated that the distorted anthracene geometry is likely the major contributor to the anomalous reactivity of 1.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.