Modulating intracellular acidification by regulating the incubation time of proton caged compounds

Eur Biophys J. 2016 Sep;45(6):565-71. doi: 10.1007/s00249-016-1122-5. Epub 2016 Mar 26.

Abstract

A proton caged compound, the 1-(2-nitrophenyl)- ethylhexadecyl sulfonate (HDNS), was dosed into HEK-293 at different incubation times. Samples were irradiated with filtered UV light for inducing photolysis of the HDNS and then probed by infrared spectroscopy. The intracellular acidification reaction can be followed by monitoring the consequent CO2 peak intensity variation. The total CO2 produced is similar for all the samples, hence it is only a function of the initial HDNS concentration. The way it is achieved, though, is different for the different incubation times and follows kinetics, which results in a combination of a linear CO2 increase and a steep CO2 increase followed by a decay. This is interpreted in terms of confinement of the HDNS into intracellular vesicles of variable average size and sensitive to UV light when they reach critical dimensions.

Keywords: CO2 monitoring; Intracellular acidification; Proton caged compounds.

MeSH terms

  • Carbon Dioxide / chemistry
  • Carbon Dioxide / metabolism
  • HEK293 Cells
  • Humans
  • Hydrogen-Ion Concentration
  • Intracellular Space / chemistry*
  • Intracellular Space / drug effects*
  • Intracellular Space / metabolism
  • Protons*
  • Sulfonic Acids / pharmacology*

Substances

  • 1-(2-nitrophenyl)-ethylhexadecylsulfonate
  • Protons
  • Sulfonic Acids
  • Carbon Dioxide