Rhamnetin induces sensitization of hepatocellular carcinoma cells to a small molecular kinase inhibitor or chemotherapeutic agents

Biochim Biophys Acta. 2016 Jul;1860(7):1417-30. doi: 10.1016/j.bbagen.2016.04.007. Epub 2016 Apr 14.

Abstract

Background: The rapid development of multi-drug resistance (MDR) process has hindered the effectiveness of advanced hepatocellular carcinoma (HCC) treatments. Notch-1 pathway, which mediates the stress-response, promotes cell survival, EMT (epithelial-mesenchymal transition) process and induces anti-apoptosis in cancer cells, would be a potential target for overcoming MDR process. This study investigated the potential application of rhamnetin, a specific inhibitor of Notch-1 pathway, in anti-tumor drug sensitization of HCC treatment.

Methods: The expression of miR-34a, proteins belonging to Notch-1 signaling pathway or MDR-related proteins was detected by quantitative polymerase chain reaction (qPCR) and western blot assay. To identify whether rhamnetin induces the chemotherapeutic sensitization in HCC cells, the MTT-assays, flow cytometry, soft agar, trans-well and nude mice assays were performed.

Results: The endogenous expression of miR-34a was significantly increased and the expression of Notch-1 and Survivin was downregulated after rhamnetin treatment. Treatment of rhamnetin also reduced the expression of MDR related proteins P-GP (P-glycoprotein) and BCRP (breast cancer resistance protein). Rhamnetin increased the susceptibility of HCC cells and especially HepG2/ADR, a MDR HCC cell line, to a small molecular kinase inhibitor sorafenib or chemotherapeutic drugs etoposide and paclitaxel. The IC(50) value of those drugs correspondingly decreased.

Conclusions: Together, our findings suggest that rhamnetin treatment may attenuate the MDR process in HCC cells. These findings may contribute to more effective strategies for HCC therapy.

General significance: Rhamnetin acts as a promising sensitizer to chemotherapy and may be a novel approach to overcome the MDR process of HCC.

Keywords: HCC; MDR; MDR-related proteins; MiR-34a; Notch-1 pathway; Rhamnetin.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Antineoplastic Agents, Phytogenic / pharmacology*
  • Antineoplastic Combined Chemotherapy Protocols / pharmacology*
  • Carcinoma, Hepatocellular / drug therapy*
  • Carcinoma, Hepatocellular / enzymology
  • Carcinoma, Hepatocellular / genetics
  • Carcinoma, Hepatocellular / pathology
  • Cell Survival / drug effects
  • Dose-Response Relationship, Drug
  • Drug Resistance, Neoplasm / drug effects*
  • Drug Resistance, Neoplasm / genetics
  • Etoposide / pharmacology*
  • Gene Expression Regulation, Neoplastic
  • Hep G2 Cells
  • Humans
  • Inhibitory Concentration 50
  • Liver Neoplasms / drug therapy*
  • Liver Neoplasms / enzymology
  • Liver Neoplasms / genetics
  • Liver Neoplasms / pathology
  • Male
  • Mice, SCID
  • MicroRNAs / genetics
  • MicroRNAs / metabolism
  • Niacinamide / analogs & derivatives*
  • Niacinamide / pharmacology
  • Paclitaxel / pharmacology*
  • Phenylurea Compounds / pharmacology*
  • Protein Kinase Inhibitors / pharmacology*
  • Quercetin / analogs & derivatives*
  • Quercetin / pharmacology
  • Receptor, Notch1 / antagonists & inhibitors
  • Receptor, Notch1 / metabolism
  • Signal Transduction / drug effects
  • Sorafenib
  • Transfection
  • Xenograft Model Antitumor Assays

Substances

  • Antineoplastic Agents, Phytogenic
  • MIRN34 microRNA, human
  • MicroRNAs
  • NOTCH1 protein, human
  • Phenylurea Compounds
  • Protein Kinase Inhibitors
  • Receptor, Notch1
  • Niacinamide
  • Etoposide
  • rhamnetin
  • Quercetin
  • Sorafenib
  • Paclitaxel