Label-free detection of DNA single-base mismatches using a simple reflectance-based optical technique

Phys Chem Chem Phys. 2016 May 21;18(19):13395-402. doi: 10.1039/c5cp08017g. Epub 2016 Apr 28.

Abstract

Rapid and quantitative detection of the binding of nucleic acids to surface-immobilized probes remains a challenge in many biomedical applications. We investigated the hybridization of a set of fully complementary and defected 12-base long DNA oligomers by using the Reflective Phantom Interface (RPI), a recently developed multiplexed label-free detection technique. Based on the simple measurement of reflected light intensity, this technology enables to quantify the hybridization directly as it occurs on the surface with a sensitivity of 10 pg mm(-2). We found a strong effect of single-base mismatches and of their location on hybridization kinetics and equilibrium binding. In line with previous studies, we found that DNA-DNA binding is weaker on a surface than in the bulk. Our data indicate that this effect is a consequence of weak nonspecific binding of the probes to the surface.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Base Pair Mismatch
  • Biosensing Techniques
  • DNA / chemistry*
  • DNA Probes / chemistry
  • Kinetics
  • Light
  • Nucleic Acid Hybridization

Substances

  • DNA Probes
  • DNA