Lewis acid-base interactions between platinum(ii) diaryl complexes and bis(perfluorophenyl)zinc: strongly accelerated reductive elimination induced by a Z-type ligand

Chem Commun (Camb). 2016 May 19;52(43):7039-42. doi: 10.1039/c6cc02433e.

Abstract

Z-type interactions between bis(perfluorophenyl)zinc and platinum(ii) diaryl complexes supported by 1,10-phenanthroline (phen), 2,2'-bipyridine (bpy), and bis(dimethylphosphino)ethane (dmpe) ligands are reported. In the solid state, the nature of the Pt-Zn interaction depends on the bidentate ligand; the phen-supported complex exhibits an unsupported Pt-Zn bond, while the dmpe derivative features additional bridging aryl interactions. A strongly accelerated rate of reductive elimination is observed for phen- and bpy-supported complexes, while aryl exchange between Pt and Zn is observed for the dmpe complex.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • 2,2'-Dipyridyl / chemistry
  • Coordination Complexes / chemistry*
  • Crystallography, X-Ray
  • Lewis Acids / chemistry*
  • Lewis Bases / chemistry*
  • Ligands
  • Models, Chemical
  • Oxidation-Reduction
  • Phenanthrolines / chemistry
  • Phosphines / chemistry
  • Proton Magnetic Resonance Spectroscopy
  • Zinc / chemistry*

Substances

  • Coordination Complexes
  • Lewis Acids
  • Lewis Bases
  • Ligands
  • Phenanthrolines
  • Phosphines
  • 2,2'-Dipyridyl
  • Zinc