An overview of rapamycin: from discovery to future perspectives

J Ind Microbiol Biotechnol. 2017 May;44(4-5):537-553. doi: 10.1007/s10295-016-1834-7. Epub 2016 Sep 9.

Abstract

Rapamycin is an immunosuppressive metabolite produced from several actinomycete species. Besides its immunosuppressive activity, rapamycin and its analogs have additional therapeutic potentials, including antifungal, antitumor, neuroprotective/neuroregenerative, and lifespan extension activities. The core structure of rapamycin is derived from (4R,5R)-4,5-dihydrocyclohex-1-ene-carboxylic acid that is extended by polyketide synthase. The resulting linear polyketide chain is cyclized by incorporating pipecolate and further decorated by post-PKS modification enzymes. Herein, we review the discovery and biological activities of rapamycin as well as its mechanism of action, mechanistic target, biosynthesis, and regulation. In addition, we introduce the many efforts directed at enhancing the production of rapamycin and generating diverse analogs and also explore future perspectives in rapamycin research. This review will also emphasize the remarkable pilot studies on the biosynthesis and production improvement of rapamycin by Dr. Demain, one of the world's distinguished scientists in industrial microbiology and biotechnology.

Keywords: Biological activity; Biosynthesis; Mechanism of action; Production enhancement; Rapamycin.

Publication types

  • Review

MeSH terms

  • Immunosuppressive Agents / chemistry
  • Immunosuppressive Agents / pharmacology
  • Mechanistic Target of Rapamycin Complex 1 / genetics
  • Mechanistic Target of Rapamycin Complex 1 / metabolism
  • Protein Conformation
  • Sirolimus / chemistry*
  • Sirolimus / pharmacology*
  • Streptomyces / metabolism
  • TOR Serine-Threonine Kinases / genetics
  • TOR Serine-Threonine Kinases / metabolism

Substances

  • Immunosuppressive Agents
  • Mechanistic Target of Rapamycin Complex 1
  • TOR Serine-Threonine Kinases
  • Sirolimus