Synthesis of monodisperse core shell PVA@P(AMPS-co-NIPAm) nanogels structured for pre-concentration of Fe(III) ions

Environ Technol. 2017 Apr;38(8):967-978. doi: 10.1080/09593330.2016.1215351. Epub 2016 Oct 2.

Abstract

Core shell-structured poly(vinyl alcohol) @ poly(2-acrylamido-2-methyl-1-propane-sulfonic acid-co-N-isopropylacrylamide) PVA@P(AMPS-co-NIPAm) spheres are synthesized. The well-defined PVA@P(AMPS-co-NIPAm) core shell nanogels with diameter nearly 30 nm enriches Fe(III), and the nanogels are characterized by FT-IR, TEM, SEM and X-ray diffraction (XRD). The many factors affecting adsorption were successfully investigated. The maximum capacity of Fe(III) ions was 320 (mg/g) for PVA@P(90AMPS-co-10NIPAm) (wt.: wt%). The equilibrium data matching well with the Langmuir model and the pseudo-second-order form described the adsorption process better than the pseudo-first-order model. Findings of the present study highlight using a simple synthesis of PVA@P(AMPS-co-NIPAm) nanogels as superior and recyclable nanoadsorbents.

Keywords: AMPS; Fe(III); Nanogels; adsorption; analytical application.

MeSH terms

  • Acrylic Resins / chemistry*
  • Adsorption
  • Chemistry Techniques, Analytical
  • Epichlorohydrin / chemistry
  • Ferric Compounds / chemistry*
  • Hydrogels / chemistry
  • Hydrogen-Ion Concentration
  • Ions
  • Microscopy, Electron, Scanning
  • Microscopy, Electron, Transmission
  • Nanogels
  • Polyethylene Glycols / chemistry*
  • Polyethyleneimine / chemistry*
  • Polyvinyl Alcohol / chemical synthesis*
  • Polyvinyl Alcohol / chemistry
  • Spectroscopy, Fourier Transform Infrared
  • Temperature
  • Waste Disposal, Fluid / methods
  • Water Pollutants, Chemical / chemistry
  • Water Purification / methods
  • X-Ray Diffraction

Substances

  • Acrylic Resins
  • Ferric Compounds
  • Hydrogels
  • Ions
  • Nanogels
  • Water Pollutants, Chemical
  • poly(2-acrylamido-2-methyl-1-propanesulfonic acid-co-N-isopropylacrylamide)
  • polyethylene glycol polyethyleneimine nanogel
  • Epichlorohydrin
  • Polyethylene Glycols
  • Polyvinyl Alcohol
  • Polyethyleneimine