Structure of the essential Haemophilus influenzae UDP-diacylglucosamine pyrophosphohydrolase LpxH in lipid A biosynthesis

Nat Microbiol. 2016 Aug 15;1(11):16154. doi: 10.1038/nmicrobiol.2016.154.

Abstract

In most Gram-negative pathogens, the hydrolysis of UDP-2,3-diacylglucosamine to generate lipid X in lipid A biosynthesis is catalysed by the membrane-associated enzyme LpxH. We report the crystal structure of LpxH in complex with its product, lipid X, unveiling a unique insertion lid above the conserved architecture of calcineurin-like phosphoesterases. This structure reveals elaborate interactions surrounding lipid X and provides molecular insights into the substrate selectivity, catalysis and inhibition of LpxH.

MeSH terms

  • Biocatalysis
  • Carbohydrate Metabolism
  • Crystallization
  • Crystallography, X-Ray
  • Glycolipids / chemistry*
  • Haemophilus influenzae / enzymology*
  • Haemophilus influenzae / metabolism
  • Hydrolysis
  • Lipid A / biosynthesis*
  • Models, Molecular
  • Pyrophosphatases / antagonists & inhibitors
  • Pyrophosphatases / chemistry*
  • Pyrophosphatases / metabolism*
  • Substrate Specificity

Substances

  • Glycolipids
  • Lipid A
  • lipid X
  • Pyrophosphatases