Structural, vibrational, and electronic properties of BaReH9 under pressure

J Phys Condens Matter. 2016 Dec 21;28(50):505701. doi: 10.1088/0953-8984/28/50/505701. Epub 2016 Oct 28.

Abstract

We present a study of the high-pressure behavior of BaReH9, a novel hydrogen-rich compound, using optical, Raman, and infrared spectroscopy as well as synchrotron x-ray diffraction. The x-ray diffraction measurements demonstrate that BaReH9 retains its hexagonal structure on room temperature compression up to 40 GPa. Optical absorption shows the absence of a gap closure to 80 GPa. Raman and IR spectra reveal the pressure evolution of a newly observed phonon peak, and large peak broadening with increasing pressure. These data constrain the disorder present in the material following the P-T paths explored.

Publication types

  • Research Support, U.S. Gov't, Non-P.H.S.
  • Research Support, Non-U.S. Gov't