Enhancement of the in vitro and in vivo antitumor activities of phosphorylated mitomycin C and etoposide derivatives by monoclonal antibody-alkaline phosphatase conjugates

Cancer Res. 1989 Nov 1;49(21):5789-92.

Abstract

Alkaline phosphatase (AP) was covalently linked to the two antitumor monoclonal antibodies, L6 (anticarcinoma) and 1F5 (anti-B lymphoma), forming conjugates that could bind to antigen-positive tumor cells. The conjugates were able to convert the prodrugs, mitomycin phosphate (MOP) and etoposide phosphate (EP), into an active mitomycin C derivative, mitomycin alcohol, and etoposide, respectively. MOP and EP were less toxic to cultured cells from the H2981 lung adenocarcinoma than their respective hydrolysis products, mitomycin alcohol and etoposide, by a factor greater than 100, and they were also less toxic in mice. Pretreatment of H2981 cells with L6-AP greatly enhanced the cytotoxic effects of MOP and EP, while 1F5-AP caused no such enhancement. A strong antitumor response was observed in H2981-bearing mice that were treated with L6-AP followed 24 h later by either MOP or a combination of MOP and EP. This response was superior to that of MOP or combinations of MOP and EP given alone.

MeSH terms

  • Adenocarcinoma / drug therapy*
  • Adenocarcinoma / pathology
  • Alkaline Phosphatase / metabolism
  • Alkaline Phosphatase / therapeutic use*
  • Animals
  • Antibodies, Monoclonal / therapeutic use
  • Biotransformation
  • Etoposide / analogs & derivatives*
  • Etoposide / metabolism
  • Etoposide / pharmacology
  • Etoposide / therapeutic use
  • Female
  • Humans
  • Lung Neoplasms / drug therapy*
  • Lung Neoplasms / pathology
  • Mice
  • Mice, Nude
  • Mitomycins / metabolism
  • Mitomycins / pharmacology
  • Mitomycins / therapeutic use*
  • Neoplasm Transplantation
  • Organophosphorus Compounds*
  • Transplantation, Heterologous
  • Tumor Cells, Cultured / cytology*
  • Tumor Cells, Cultured / drug effects

Substances

  • Antibodies, Monoclonal
  • Mitomycins
  • Organophosphorus Compounds
  • mitomycin phosphate
  • etoposide phosphate
  • Etoposide
  • Alkaline Phosphatase