Comparative hepatotoxicity of 6:2 fluorotelomer carboxylic acid and 6:2 fluorotelomer sulfonic acid, two fluorinated alternatives to long-chain perfluoroalkyl acids, on adult male mice

Arch Toxicol. 2017 Aug;91(8):2909-2919. doi: 10.1007/s00204-016-1917-2. Epub 2016 Dec 28.

Abstract

Due to their structural similarities, 6:2 fluorotelomer sulfonic acid (6:2 FTSA) and 6:2 fluorotelomer carboxylic acid (6:2 FTCA) are often used as alternatives to perfluorooctane sulfonate (PFOS) and perfluorooctanoic acid (PFOA), respectively. With limited health risk data and 6:2 FTSA detection in water and sludge, the toxicity of these chemicals is of growing concern. Here, adult male mice were exposed with 5 mg/kg/day of 6:2 FTCA or 6:2 FTSA for 28 days to investigate their hepatotoxicological effects. In contrast to 6:2 FTCA, 6:2 FTSA was detected at high and very high levels in serum and liver, respectively, demonstrating bioaccumulation potential and slow elimination. Furthermore, 6:2 FTSA induced liver weight increase, inflammation, and necrosis, whereas 6:2 FTCA caused no obvious liver injury, with fewer significantly altered genes detected compared with that of 6:2 FTSA (39 vs. 412). Although PFOA and PFOS commonly activate peroxisome proliferator-activated receptor α (PPARα), 6:2 FTSA induced an increase in PPARγ and related proteins, but not in lipid metabolism-related genes such as PPARα. Our results showed that 6:2 FTCA and 6:2 FTSA exhibited weak and moderate hepatotoxicity, respectively, compared with that reported for legacies PFOA and PFOS.

Keywords: 6:2 FTCA; 6:2 FTSA; Comparative hepatotoxicity; PFAAs alternatives.

Publication types

  • Comparative Study

MeSH terms

  • Alkanesulfonic Acids / toxicity
  • Animals
  • Caprylates / toxicity
  • Carboxylic Acids / toxicity*
  • Chemical and Drug Induced Liver Injury / etiology*
  • Fluorocarbons / toxicity
  • Lipid Metabolism
  • Liver / drug effects*
  • Male
  • Mice
  • Organ Size / drug effects
  • PPAR alpha / metabolism
  • PPAR gamma / metabolism
  • Sulfonic Acids / toxicity*

Substances

  • Alkanesulfonic Acids
  • Caprylates
  • Carboxylic Acids
  • Fluorocarbons
  • PPAR alpha
  • PPAR gamma
  • Sulfonic Acids
  • perfluorooctanoic acid
  • perfluorooctane sulfonic acid