Near-Infrared Fluorescent Ag2 Se-Cetuximab Nanoprobes for Targeted Imaging and Therapy of Cancer

Small. 2017 Jan;13(3). doi: 10.1002/smll.201602309. Epub 2016 Nov 7.

Abstract

Theranostic nanoprobes integrated with diagnostic imaging and therapy capabilities have shown great potential for highly effective tumor therapy by realizing imaging-guided drug delivery and tumor treatment. Developing novel high-performance nanoprobes is an important basis for tumor theranostic application. Here, near-infrared (NIR) fluorescent and low-biotoxicity Ag2 Se quantum dots (QDs) have been coupled with cetuximab, a clinical antiepidermal growth factor receptor antibody drug for tumor therapy, via a facile bioconjugation strategy to prepare multifunctional Ag2 Se-cetuximab nanoprobes. Compared with the Ag2 Se QDs alone, the Ag2 Se-cetuximab nanoprobes display faster and more enrichment at the site of orthotopic tongue cancer, and thus present better NIR fluorescence contrast between the tumor and the surrounding regions. At 24 h postinjection, the NIR fluorescence of Ag2 Se-cetuximab nanoprobes at the tumor site is still easily detectable, whereas no fluorescence is observed for the Ag2 Se QDs. Moreover, the Ag2 Se-cetuximab nanoprobes have also significantly inhibited the tumor growth and improved the survival rate of orthotopic tongue cancer-bearing nude mice from 0% to 57.1%. Taken together, the constructed multifunctional Ag2 Se-cetuximab nanoprobes have achieved combined targeted imaging and therapy of orthotopic tongue cancer, which may greatly contribute to the development of nanotheranostics.

Keywords: cancer therapy; cetuximab; targeted imaging; theranostic nanoprobes; tumor therapy.

MeSH terms

  • Animals
  • Cell Death / drug effects
  • Cell Line
  • Cetuximab / therapeutic use*
  • Diagnostic Imaging*
  • Female
  • Fluorescence
  • Humans
  • Hydrophobic and Hydrophilic Interactions
  • Infrared Rays*
  • Mice, Inbred BALB C
  • Nanoparticles / chemistry*
  • Quantum Dots / ultrastructure
  • Selenium Compounds / chemistry*
  • Selenium Compounds / toxicity
  • Silver / chemistry*
  • Silver / toxicity
  • Solubility
  • Surface Properties
  • Survival Analysis
  • Theranostic Nanomedicine
  • Time Factors
  • Tongue Neoplasms / diagnosis*
  • Tongue Neoplasms / drug therapy*
  • Tongue Neoplasms / pathology
  • Treatment Outcome
  • Water / chemistry

Substances

  • Selenium Compounds
  • Water
  • Silver
  • Cetuximab