Magnetic resonance spectroscopy of an atomically thin material using a single-spin qubit

I Lovchinsky; J D Sanchez-Yamagishi; E K Urbach; S Choi; S Fang; T I Andersen; K Watanabe; T Taniguchi; A Bylinskii; E Kaxiras; P Kim; H Park; M D Lukin

doi:10.1126/science.aal2538

Magnetic resonance spectroscopy of an atomically thin material using a single-spin qubit

Science. 2017 Feb 3;355(6324):503-507. doi: 10.1126/science.aal2538. Epub 2017 Jan 19.

Authors

I Lovchinsky¹, J D Sanchez-Yamagishi^{1

2}, E K Urbach¹, S Choi¹, S Fang¹, T I Andersen¹, K Watanabe³, T Taniguchi³, A Bylinskii^{1

2}, E Kaxiras^{1

4}, P Kim¹, H Park^{5

2

6}, M D Lukin⁵

Affiliations

¹ Department of Physics, Harvard University, Cambridge, MA 02138, USA.
² Department of Chemistry and Chemical Biology, Harvard University, Cambridge, MA 02138, USA.
³ National Institute for Materials Science, Tsukuba, Japan.
⁴ John A. Paulson School of Engineering and Applied Sciences, Harvard University, Cambridge, MA 02138, USA.
⁵ Department of Physics, Harvard University, Cambridge, MA 02138, USA. [email protected] [email protected].
⁶ Broad Institute of MIT and Harvard, 7 Cambridge Center, Cambridge, MA 02142, USA.

PMID: 28104795
DOI: 10.1126/science.aal2538

Abstract

Two-dimensional (2D) materials offer a promising platform for exploring condensed matter phenomena and developing technological applications. However, the reduction of material dimensions to the atomic scale poses a challenge for traditional measurement and interfacing techniques that typically couple to macroscopic observables. We demonstrate a method for probing the properties of 2D materials via nanometer-scale nuclear quadrupole resonance (NQR) spectroscopy using individual atomlike impurities in diamond. Coherent manipulation of shallow nitrogen-vacancy (NV) color centers enables the probing of nanoscale ensembles down to approximately 30 nuclear spins in atomically thin hexagonal boron nitride (h-BN). The characterization of low-dimensional nanoscale materials could enable the development of new quantum hybrid systems, combining atomlike systems coherently coupled with individual atoms in 2D materials.

Publication types

Research Support, Non-U.S. Gov't