Elucidating light-induced charge accumulation in an artificial analogue of methane monooxygenase enzymes using time-resolved X-ray absorption spectroscopy

Chem Commun (Camb). 2017 Feb 28;53(18):2725-2728. doi: 10.1039/c6cc08748e.

Abstract

We report the use of time-resolved X-ray absorption spectroscopy in the ns-μs time scale to track the light induced two electron transfer processes in a multi-component photocatalytic system, consisting of [Ru(bpy)3]2+/ a diiron(iii,iii) model/triethylamine. EXAFS analysis with DFT calculations confirms the structural configurations of the diiron(iii,iii) and reduced diiron(ii,ii) states.