Novel fluorene-based supramolecular sensor for selective detection of amoxicillin in water and blood

Ecotoxicol Environ Saf. 2017 Jul:141:25-29. doi: 10.1016/j.ecoenv.2017.03.003. Epub 2017 Mar 12.

Abstract

Synthesis, characterization and molecular recognition properties of fluorene based supramolecular cleft 1 is reported. The cleft molecule 1 was prepared in a single-step with good yield (85% yield), by linking Fluorene with 1-ethyl piperazine. The cleft molecule 1 was carefully characterized using various spectroscopic techniques such as NMR and mass spectrometry. The supramolecular interaction of cleft 1 with amoxicillin, 6APA, aspirin, captopril, cefotaxime, ceftriaxone, cefuroxime, diclofenac, penicillin, and cephradine was evaluated by fluorescent spectroscopy. The molecular recognition studies showed that amoxicillin selectively binds with cleft 1 in the presence of other drugs. The analytical method developed for the supramolecular interaction of molecular cleft 1 and amoxicillin was validated at varying pH, concentration and temperature during recognition process. Job's plots indicated that the stochiometry of the interactions between the cleft 1 and the amoxicillin was 1:1.

Keywords: Amoxicillin; Fluorescence spectroscopy; Molecular recognition; Supramolecular hosts.

MeSH terms

  • Amoxicillin / analysis*
  • Amoxicillin / blood
  • Anti-Bacterial Agents / analysis*
  • Anti-Bacterial Agents / blood
  • Fluorenes / chemistry*
  • Humans
  • In Vitro Techniques
  • Magnetic Resonance Spectroscopy
  • Models, Theoretical
  • Piperazines / chemistry*
  • Sensitivity and Specificity
  • Spectrometry, Fluorescence
  • Temperature
  • Water Pollutants, Chemical / analysis*
  • Water Pollutants, Chemical / blood

Substances

  • Anti-Bacterial Agents
  • Fluorenes
  • Piperazines
  • Water Pollutants, Chemical
  • Amoxicillin