Abstract
When cells are exposed to heat shock and various other stresses, heat shock factor 1 (HSF1) is activated, and the heat shock response (HSR) is elicited. To better understand the molecular regulation of the HSR, we used 2D-PAGE-based proteome analysis to screen for heat shock-induced post-translationally modified cellular proteins. Our analysis revealed that two protein spots typically present on 2D-PAGE gels and containing heterogeneous nuclear ribonucleoprotein K (hnRNP K) with trioxidized Cys132 disappeared after the heat shock treatment and reappeared during recovery, but the total amount of hnRNP K protein remained unchanged. We next tested whether hnRNP K plays a role in HSR by regulating HSF1 and found that hnRNP K inhibits HSF1 activity, resulting in reduced expression of hsp70 and hsp27 mRNAs. hnRNP K also reduced binding affinity of HSF1 to the heat shock element by directly interacting with HSF1 but did not affect HSF1 phosphorylation-dependent activation or nuclear localization. hnRNP K lost its ability to induce these effects when its Cys132 was substituted with Ser, Asp, or Glu. These findings suggest that hnRNP K inhibits transcriptional activity of HSF1 by inhibiting its binding to heat shock element and that the oxidation status of Cys132 in hnRNP K is critical for this inhibition.
Keywords:
Heat shock factor protein 1 (HSF1); heat shock protein (HSP); hnRNP K; mass spectrometry (MS); post-translational modification (PTM); proteomics; redox regulation.
© 2017 by The American Society for Biochemistry and Molecular Biology, Inc.
MeSH terms
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Amino Acid Substitution
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Animals
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Cell Line, Tumor
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Cystine / metabolism
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DNA-Binding Proteins / antagonists & inhibitors*
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DNA-Binding Proteins / genetics
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DNA-Binding Proteins / metabolism
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Gene Expression Profiling
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Gene Expression Regulation*
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HEK293 Cells
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HSP27 Heat-Shock Proteins / antagonists & inhibitors*
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HSP27 Heat-Shock Proteins / genetics
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HSP27 Heat-Shock Proteins / metabolism
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HSP70 Heat-Shock Proteins / antagonists & inhibitors*
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HSP70 Heat-Shock Proteins / genetics
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HSP70 Heat-Shock Proteins / metabolism
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Heat Shock Transcription Factors
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Heat-Shock Proteins
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Heterogeneous-Nuclear Ribonucleoprotein K / antagonists & inhibitors
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Heterogeneous-Nuclear Ribonucleoprotein K / genetics
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Heterogeneous-Nuclear Ribonucleoprotein K / metabolism*
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Hot Temperature / adverse effects
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Humans
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Mice
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Molecular Chaperones
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Mutation
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Oxidation-Reduction
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Protein Processing, Post-Translational*
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RNA Interference
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RNA, Messenger / metabolism
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Recombinant Fusion Proteins / chemistry
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Recombinant Fusion Proteins / genetics
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Recombinant Fusion Proteins / metabolism
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Response Elements*
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Ribonucleoproteins / antagonists & inhibitors
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Ribonucleoproteins / genetics
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Ribonucleoproteins / metabolism
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Transcription Factors / antagonists & inhibitors*
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Transcription Factors / genetics
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Transcription Factors / metabolism
Substances
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DNA-Binding Proteins
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HSF1 protein, human
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HSP27 Heat-Shock Proteins
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HSP70 Heat-Shock Proteins
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HSPB1 protein, human
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Heat Shock Transcription Factors
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Heat-Shock Proteins
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Heterogeneous-Nuclear Ribonucleoprotein K
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Molecular Chaperones
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RNA, Messenger
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Recombinant Fusion Proteins
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Ribonucleoproteins
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Transcription Factors
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HNRNPK protein, human
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Cystine