Micro-matrix solid-phase dispersion coupled with MEEKC for quantitative analysis of lignans in Schisandrae Chinensis Fructus using molecular sieve TS-1 as a sorbent

J Chromatogr B Analyt Technol Biomed Life Sci. 2017 Sep 15:1063:174-179. doi: 10.1016/j.jchromb.2017.08.024. Epub 2017 Aug 24.

Abstract

A simple and effective method was developed for determining lignans in Schisandrae Chinensis Fructus by using a micro-matrix solid phase dispersion (MSPD) technique coupled with microemulsion electrokinetic chromatography (MEEKC). Molecular sieve, TS-1, was applied as a solid supporting material in micro MSPD extraction for the first time. Parameters that affect extraction efficiency, such as type of dispersant, mass ratio of the sample to the dispersant, grinding time, elution solvent and volume were optimized. The optimal extraction conditions involve dispersing 25mg of powdered Schisandrae samples with 50mg of TS-1 by a mortar and pestle. A grinding time of 150s was adopted. The blend was then transferred to a solid-phase extraction cartridge and the target analytes were eluted with 500μL of methanol. Moreover, several parameters affecting MEEKC separation were studied, including the type of oil, SDS concentration, type and concentration of cosurfactant, and concentration of organic modifier. A satisfactory linearity (R>0.9998) was obtained, and the calculated limits of quantitation were less than 2.77μg/mL. Finally, the micro MSPD-MEEKC method was successfully applied to the analysis of lignans in complex Schisandrae fructus samples.

Keywords: Lignans; Micro matrix solid-phase dispersion; Microemulsion electrokinetic chromatography; Molecular sieve; Schisandra.

MeSH terms

  • Chromatography, Micellar Electrokinetic Capillary / methods*
  • Fruit / chemistry*
  • Lignans / analysis*
  • Lignans / chemistry
  • Lignans / isolation & purification
  • Linear Models
  • Methanol
  • Plant Extracts
  • Reproducibility of Results
  • Schisandra / chemistry*
  • Sensitivity and Specificity
  • Silicates / chemistry
  • Solid Phase Extraction / methods*
  • Surface-Active Agents
  • Titanium / chemistry

Substances

  • Lignans
  • Plant Extracts
  • Silicates
  • Surface-Active Agents
  • titanium silicide
  • Titanium
  • Methanol