To enable high-speed long-distance underwater optical wireless communication (UOWC) supplementing traditional underwater wireless communication, a low-power 520 nm green laser diode (LD) based UOWC system was proposed and experimentally demonstrated to implement maximal communication capacity of up to 2.70 Gbps data rate over a 34.5 m underwater transmission distance by using non-return-to-zero on-off keying (NRZ-OOK) modulation scheme. Moreover, maximum data rates of up to 4.60 Gbps, 4.20 Gbps, 3.93 Gbps, 3.88 Gbps, and 3.48 Gbps at underwater distances of 2.3 m, 6.9 m, 11.5 m, 16.1 m and 20.7 m were achieved, respectively. The light attenuation coefficient of ~0.44 dB/m was obtained and the beam divergence angle is 0.35°, so the aallowable underwater transmission distance can be estimated to be ~90.7 m at a data rate of 0.15 Gbps with a corresponding received light-output power of -33.01 dBm and a bit-error rate (BER) of 2.0 ×10-6. In addition, when the data rate is up to 1 Gbps, the UOWC distance is predicted to be ~62.7 m for our proposed UOWC system. The achievements we make are suitable for applications requiring high-speed long-distance real-time UOWC.