Nano-rod Ca-decorated sludge derived carbon for removal of phosphorus

Environ Pollut. 2018 Feb:233:698-705. doi: 10.1016/j.envpol.2017.10.099. Epub 2017 Nov 6.

Abstract

Recovering phosphorus (P) from waste streams takes the unique advantage in simultaneously addressing the crisis of eutrophication and the shortage of P resource. A novel calcium decorated sludge carbon (Ca-SC) was developed from dyeing industry wastewater treatment sludge by decorating calcium (Ca) to effectively adsorb phosphorus from solution. The X-ray diffraction (XRD) and Fourier transform infrared (FTIR) techniques were used to characterize the Ca-SCs, followed by isotherm and kinetic sorption experiments. A preferred design with CaCO3 to sludge mass ratio of 1:2 was found to have a sorption capacity of 116.82 mg/g for phosphorus. This work reveals the crucial role of well-dispersed nano-rod calcium on the Ca-SC surface for the sorption of phosphorus. Moreover, the decoration of nano-rod calcium was found to further promote the uptake of phosphorus through the formation of hydroxylapatite (Ca5(PO4)3(OH)). Thus, the development of decorated Ca-SC for sorption of phosphorus is very important in solving the P pollution and resource loss.

Keywords: Ca decorated sludge carbon; Crystallization; Phosphorus; Sorption.

MeSH terms

  • Adsorption
  • Calcium / chemistry*
  • Carbon / chemistry*
  • Kinetics
  • Nanostructures / chemistry*
  • Phosphorus / analysis
  • Phosphorus / chemistry*
  • Sewage
  • Waste Disposal, Fluid / methods*
  • Wastewater / chemistry
  • X-Ray Diffraction

Substances

  • Sewage
  • Waste Water
  • Phosphorus
  • Carbon
  • Calcium