Serum paracetamol-protein adducts in ambulatory subjects: Relationship to recent reported paracetamol use

Biomarkers. 2018 May;23(3):288-292. doi: 10.1080/1354750X.2017.1410857. Epub 2017 Dec 8.

Abstract

Context: Serum paracetamol-protein adducts (PPAs) are a novel potential biomarker of paracetamol exposure. The relationship between serum PPA concentrations and reported paracetamol use in ambulatory adults has not been previously described.

Materials and methods: This was a cross-sectional study of ambulatory adults. A detailed medication history was obtained from all subjects and subjects were stratified by reported paracetamol use in the 2 weeks prior to enrolment. Serum PPAs were measured in all subjects and correlated with reported dose, time of last ingestion and demographics.

Results: We enrolled 230 in the paracetamol exposure arm and 74 in the no exposure arm. 98/230 (42.6%)of subjects who reported paracetamol exposure had PPA detected and 68/74 (91.9%) of subjects who denied paracetamol exposure had no PPA detected. PPA concentrations were positively correlated with total paracetamol dose and with more recent ingestion.

Discussion: Detection of serum PPA generally reflects paracetamol exposure histories in ambulatory adults. Concentrations are well correlated with reported dose and time from last dose.

Conclusions: Serum PPA can be detected with reported therapeutic use of paracetamol but may not be detected in all patients who report taking paracetamol.

Keywords: APAP-CYS; Paracetamol; overdose; protein adducts.

MeSH terms

  • Acetaminophen / administration & dosage
  • Acetaminophen / blood
  • Acetaminophen / chemistry*
  • Acetaminophen / therapeutic use
  • Adult
  • Analgesics, Non-Narcotic
  • Blood Proteins / analysis
  • Blood Proteins / chemistry*
  • Cross-Sectional Studies
  • Dose-Response Relationship, Drug
  • Drug Overdose
  • Female
  • Humans
  • Male
  • Middle Aged
  • Walking
  • Young Adult

Substances

  • Analgesics, Non-Narcotic
  • Blood Proteins
  • Acetaminophen