Fully biodegradable Poly(lactic acid)/Starch blends: A review of toughening strategies

Int J Biol Macromol. 2018 Apr 1:109:99-113. doi: 10.1016/j.ijbiomac.2017.12.048. Epub 2017 Dec 14.

Abstract

Polylactic acid (PLA) and Starch are both bio-based biodegradable polymers that have properties that are complementary to each other. PLA/starch blend exploits the good mechanical property of PLA and the low cost of Starch. However, PLA/Starch blend is intrinsically brittle. This paper reviews the current state of arts in toughening of PLA/Starch blend, which are categorized as: Additive Plasticization, Mixture Softening, Elastomer Toughening and Interphase Compatibilization. These strategies are not mutually exclusive and can be applied jointly in a single blend, opening up a wide range of toughening techniques that can be employed in PLA/Starch blend. Even though significant progress has been made in this area, there is still much room for research, in order to achieve easy to process, fully bio-based and completely biodegradable PLA/Starch blends that have mechanical properties suitable for a wide range of applications.

Keywords: Bio-based; Biodegradable; Compatibilization; Poly(lactic acid); Starch; Sustainability; Toughening.

Publication types

  • Review

MeSH terms

  • Biocompatible Materials / chemistry*
  • Biomimetic Materials / chemistry*
  • Chemical Phenomena
  • Materials Testing
  • Mechanical Phenomena
  • Polyesters / chemistry*
  • Starch / chemistry*

Substances

  • Biocompatible Materials
  • Polyesters
  • poly(lactide)
  • Starch