Structure, kinetics, molecular and redox properties of a cytosolic and developmentally regulated fungal catalase-peroxidase

Arch Biochem Biophys. 2018 Feb 15:640:17-26. doi: 10.1016/j.abb.2017.12.021. Epub 2018 Jan 2.

Abstract

CAT-2, a cytosolic catalase-peroxidase (CP) from Neurospora crassa, which is induced during asexual spore formation, was heterologously expressed and characterized. CAT-2 had the Met-Tyr-Trp (M-Y-W) adduct required for catalase activity. Its KM for H2O2 was micromolar for peroxidase and millimolar for catalase activity. A Em = -158 mV reduction potential value was obtained and the Soret band shift suggested a mixture of low and high spin ferric iron. CAT-2 EPR spectrum at 10 K indicated an axial and a rhombic component. With peroxyacetic acid (PAA), formation of Compound I* was observed with EPR. CAT-2 homodimer crystallographic structure contained two K+ ions; Glu107 residues were displaced to bind them. CAT-2 showed the essential amino acid residues for activity in similar positions to other CPs. CAT-2 Arg426 is oriented towards the M-Y-W adduct, interacting with the deprotonated Tyr238 hydroxyl group. A perhydroxy modification of the indole nitrogen of Trp90 was oriented toward the catalytic His91. In contrast to cytochrome c peroxidase and ascorbate peroxidase, the catalase-peroxidase heme propionates are not exposed to the solvent. Together with other N. crassa enzymes that utilize H2O2 as a substrate, CAT-2 has many tryptophan and proline residues at its surface, probably related to H2O2 selection in water.

Keywords: Amino-acid radical; Catalase-peroxidase structure; Heme-EPR; Kinetics; M-Y-W adduct; Metal-binding; surface residues with increased residence time for H(2)O(2).

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Catalase / chemistry
  • Catalase / genetics
  • Catalase / metabolism*
  • Cloning, Molecular
  • Crystallography, X-Ray
  • Cytosol / enzymology*
  • Electron Spin Resonance Spectroscopy
  • Gene Expression Regulation
  • Hydrogen Peroxide / metabolism*
  • Kinetics
  • Neurospora crassa / enzymology*
  • Oxidation-Reduction
  • Peroxidases / chemistry
  • Peroxidases / metabolism*
  • Protein Conformation
  • Protein Multimerization
  • Tryptophan / metabolism
  • Tyrosine / metabolism

Substances

  • Tyrosine
  • Tryptophan
  • Hydrogen Peroxide
  • Peroxidases
  • Catalase