Interactions of dimethylaminoethyl methacrylate copolymer with non-acidic drugs demonstrated high solubilization in vitro and pronounced sustained release in vivo

Eur J Pharm Biopharm. 2018 Apr:125:68-75. doi: 10.1016/j.ejpb.2018.01.006. Epub 2018 Jan 10.

Abstract

Recent work demonstrated remarkable solubilization effects of methacrylate-copolymer Eudragit EPO (EPO) not only with acidic drugs but interestingly also with poorly soluble basic compounds. The current work studied EPO-mediated solubilization effects first in vitro using felodipine (FLP) and tamoxifen (TMX) as model compounds. EPO-containing solutions were subsequently compared in a rat pharmacokinetic study against reference solutions and suspensions. Surprisingly, solution formulations with EPO did not result in an increased relative oral bioavailability. Exposure was reduced for both drugs and plasma-profiles of the EPO solutions showed a delayed and lower maximum plasma concentration compared to the reference formulations. This sustained in vivo release was likely due to combined effects of strong drug-polymer interactions and pH-dependent precipitation of the polymer in the rat intestine. Remarkable was that in vitro drug-polymer coprecipitates did not reveal crystalline drug by polarized light microscopy. Thus, such a formulation approach provides a rather simple opportunity to modify drug release in vivo. However, this may be rather an approach for preclinical formulations, if high peak-to-trough ratios of plasma levels are problematic regarding adverse effects related to Cmax or if plasma concentrations drop too fast below required pharmacological concentrations.

Keywords: Oral bioavailability; Polymer drug interaction; Solubility enhancement; Sustained release.

MeSH terms

  • Animals
  • Delayed-Action Preparations / administration & dosage
  • Delayed-Action Preparations / metabolism
  • Dose-Response Relationship, Drug
  • Felodipine / administration & dosage
  • Felodipine / metabolism*
  • Male
  • Polymethacrylic Acids / administration & dosage
  • Polymethacrylic Acids / metabolism*
  • Rats
  • Rats, Sprague-Dawley
  • Solubility
  • Tamoxifen / administration & dosage
  • Tamoxifen / metabolism*

Substances

  • Delayed-Action Preparations
  • Polymethacrylic Acids
  • Tamoxifen
  • methylmethacrylate-methacrylic acid copolymer
  • Felodipine