Targeted versus untargeted omics - the CAFSA story

J Inherit Metab Dis. 2018 May;41(3):447-456. doi: 10.1007/s10545-017-0134-3. Epub 2018 Feb 8.

Abstract

Background: In 2009, untargeted metabolomics led to the delineation of a new clinico-biological entity called cerebellar ataxia with elevated cerebrospinal free sialic acid, or CAFSA. In order to elucidate CAFSA, we applied sequentially targeted and untargeted omic approaches.

Methods and results: First, we studied five of the six CAFSA patients initially described. Besides increased CSF free sialic acid concentrations, three patients presented with markedly decreased 5-methyltetrahydrofolate (5-MTHF) CSF concentrations. Exome sequencing identified a homozygous POLG mutation in two affected sisters, but failed to identify a causative gene in the three sporadic patients with high sialic acid but low 5-MTHF. Using targeted mass spectrometry, we confirmed that free sialic acid was increased in the CSF of a third known POLG-mutated patient. We then pursued pathophysiological analyses of CAFSA using mass spectrometry-based metabolomics on CSF from two sporadic CAFSA patients as well as 95 patients with an unexplained encephalopathy and 39 controls. This led to the identification of a common metabotype between the two initial CAFSA patients and three additional patients, including one patient with Kearns-Sayre syndrome. Metabolites of the CSF metabotype were positioned in a reconstruction of the human metabolic network, which highlighted the proximity of the metabotype with acetyl-CoA and carnitine, two key metabolites regulating mitochondrial energy homeostasis.

Conclusion: Our genetic and metabolomics analyses suggest that CAFSA is a heterogeneous entity related to mitochondrial DNA alterations either through POLG mutations or a mechanism similar to what is observed in Kearns-Sayre syndrome.

Keywords: Cerebellar ataxia; Exome; Folate; Metabolomics. Cerebrospinal fluid; Mitochondrial disease; Sialic acid.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Adult
  • Case-Control Studies
  • Cerebellar Ataxia / cerebrospinal fluid
  • Cerebellar Ataxia / diagnosis*
  • Cerebellar Ataxia / genetics
  • Cerebellar Ataxia / metabolism
  • DNA Mutational Analysis
  • DNA Polymerase gamma / genetics
  • DNA, Mitochondrial / analysis
  • Exome Sequencing / methods
  • Female
  • Genomics / methods*
  • Humans
  • Male
  • Mass Spectrometry
  • Metabolomics / methods*
  • N-Acetylneuraminic Acid / cerebrospinal fluid*
  • Siblings
  • Tetrahydrofolates / analysis
  • Tetrahydrofolates / cerebrospinal fluid*

Substances

  • DNA, Mitochondrial
  • Tetrahydrofolates
  • DNA Polymerase gamma
  • POLG protein, human
  • N-Acetylneuraminic Acid
  • 5-methyltetrahydrofolate