Simple fabrication of Chitosan/Graphene nanoplates composite spheres for efficient adsorption of acid dyes from aqueous solution

Int J Biol Macromol. 2018 Jun:112:1048-1054. doi: 10.1016/j.ijbiomac.2018.02.074. Epub 2018 Feb 13.

Abstract

A facile method for the fabrication of crosslinked chitosan/graphene nanoplates composite sphere (CS/GNPs) was presented. The obtained samples were characterized by transmission electron microscopy (TEM), X-ray diffraction (XRD), X-ray photoelectron spectroscopic (XPS) and thermogravimetric analysis (TGA). The adsorption activities of CS/GNPs for methyl orange (MO) and acid red 1 (AR1) were evaluated such as the effect of pH and GNPs content, as well as adsorption kinetics and isotherms. In view of practical, the reusability of CS/GNPs was also tested. The resulting adsorption capacity for MO is 230.91mgg-1 and 132.94mgg-1 for AR1, respectively. After saturated adsorption, CS/GNPs can be efficiently regenerated and reused with little uptake loss. Therefore, CS/GNPs is the apromising adsorbent with non-toxic, efficient, low-cost and easy to prepare for the dye removal.

Keywords: Acid dyes; Adsorption; Chitosan; Composite spheres; Graphene nanoplates.

MeSH terms

  • Acids / chemistry*
  • Adsorption
  • Azo Compounds / chemistry
  • Azo Compounds / isolation & purification
  • Chitosan / chemistry*
  • Coloring Agents / isolation & purification*
  • Graphite / chemistry*
  • Hydrogen-Ion Concentration
  • Kinetics
  • Nanospheres / chemistry*
  • Nanospheres / ultrastructure
  • Photoelectron Spectroscopy
  • Solutions
  • Temperature
  • Time Factors
  • Water / chemistry*

Substances

  • Acids
  • Azo Compounds
  • Coloring Agents
  • Solutions
  • Water
  • methyl orange
  • Graphite
  • Chitosan