Enzymatic Transition States and Drug Design

Chem Rev. 2018 Nov 28;118(22):11194-11258. doi: 10.1021/acs.chemrev.8b00369. Epub 2018 Oct 18.

Abstract

Transition state theory teaches that chemically stable mimics of enzymatic transition states will bind tightly to their cognate enzymes. Kinetic isotope effects combined with computational quantum chemistry provides enzymatic transition state information with sufficient fidelity to design transition state analogues. Examples are selected from various stages of drug development to demonstrate the application of transition state theory, inhibitor design, physicochemical characterization of transition state analogues, and their progress in drug development.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.
  • Review

MeSH terms

  • Animals
  • Drug Design*
  • Enzyme Inhibitors / chemical synthesis*
  • Enzyme Inhibitors / chemistry
  • Enzyme Inhibitors / pharmacology*
  • Enzymes / chemistry*
  • Enzymes / metabolism
  • Humans
  • Kinetics
  • Quantum Theory*

Substances

  • Enzyme Inhibitors
  • Enzymes